On my first game, I finished off Admiral Havelock when he had his gun out. The execution had Corvo stabbing the admiral through his pistol arm, turning the gun around, and forcing him to shoot himself. Wicked.
On this high chaos playthrough I'm on now, I killed the Lord Regent with an adrenaline execution. Not sure if its because I used bloodthirsty, but Corvo turned him around, stabbed him down his shoulder to hold him in place, and broke his neck.