My all time favorite line comes from the "Wizard of Oz", when the wicked witch says to Dorthy "I'll get you, my pretty... and your little dog too!!!"
And from the same movie, when Dorthy is scolding The Wizard, "You're a very bad man!"
My second would be from "LOTR: The Fellowship ...", when Gandalf and Saruman are walking in the garden at Isengard, and Saruman says to Gandalf... well, see my sig.
The third would be from "Evil Dead", when Ash fastens the chainsaw to his arm, loads his double barrel shotgun with his teeth, then snaps the breech of the shotgun closed. He looks into the camera and says "Groovy".
I laughed at that scene till I had tears in my eyes the first time I saw the movie.
Ok, what are some of yours?
