Theives Guild was my fav. Great characters, great missions, great result. My only gripe is that it could've been longer, and that some of the minor characters like Rune and Saphire were obviously meant for followers, but not enough time for that to become reality.
And its also the only questline to have a cutscene, to my knowlegde.
DB was quite good, but waaaaayyyy to short, and the majority of contracts were boring and unimaginative, unlike Oblivion's.
Companions was okay, but was a tad boring.
Dont really care for the College of Winterhold. A few quests and BANG,
i mean, really?