If you did the optional wintahold college quest, you'll know that conjuration master guy turned into a ghost after he hit the soul gem with keening. Kagrenac did something similar but on a larger scale so his whole race became the ghosts seen in morrowind and its expansion, tribunal.
Close, but no cigar.
The Dwemer endeavor was to escape the Mundus, which in their worldview is a trap, and return to the first brushstroke of Anu and Padomay, using Numidium as a tool for ascenscion.
Their plan was to reverse the flow of creation. Instead of being many smaller souls, they longed to be one big divine one again.
However, Kagrenac was rushed into completing his project too soon, the armies of the Triune were at the gates.
If he made a mistake or if something else went wrong is unknown, but when he struck the Heart he bound the entire Dwemer race to Numidium, only it did not activate.
Or possibly it did, and the Triune deactivated it before it was fully powered up.
It seems Arniel did indeed succeed in replicating the Dwemer experiments on a much smaller scale.
He uncreated himself and bound his soul to the nearest mythic recepticle, the Dovakhiin.
Were lucky he was only halfway competent, or else he might have bound the entire Breton race to the Dovakhiin.
Consensus holds that Dwemer ghosts are of those that died before Kagrenac's folly.
http://www.imperial-library.info/content/final-report-trebonius